Enhanced methane activation on diluted metal-metal ensembles under an electric field: Breakthrough in alloy catalysis

Maki Torimoto; Shuhei Ogo; Danny Harjowinoto; Takuma Higo; Jeong Gil Seo; Shinya Furukawa; Yasushi Sekine

doi:10.1039/c9cc02794g

Enhanced methane activation on diluted metal-metal ensembles under an electric field: Breakthrough in alloy catalysis

Maki Torimoto, Shuhei Ogo, Danny Harjowinoto, Takuma Higo, Jeong Gil Seo, Shinya Furukawa, Yasushi Sekine

Research output: Contribution to journal › Article › peer-review

10 Citations (Scopus)

Abstract

Methane activation on diluted metal ensembles is a challenging task in the field of alloy chemistry. This report describes that synergy between an electric field and Pd-Zn alloy allows improved catalytic activities in the steam reforming of methane. Because of surface protonics, Pd-Pd ensembles are no longer needed. Ligand effects facilitate methane conversion.

Original language	English
Pages (from-to)	6693-6695
Number of pages	3
Journal	Chemical Communications
Volume	55
Issue number	47
DOIs	https://doi.org/10.1039/c9cc02794g
Publication status	Published - 2019

ASJC Scopus subject areas

Catalysis
Electronic, Optical and Magnetic Materials
Ceramics and Composites
Chemistry(all)
Surfaces, Coatings and Films
Metals and Alloys
Materials Chemistry

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title = "Enhanced methane activation on diluted metal-metal ensembles under an electric field: Breakthrough in alloy catalysis",

abstract = "Methane activation on diluted metal ensembles is a challenging task in the field of alloy chemistry. This report describes that synergy between an electric field and Pd-Zn alloy allows improved catalytic activities in the steam reforming of methane. Because of surface protonics, Pd-Pd ensembles are no longer needed. Ligand effects facilitate methane conversion.",

author = "Maki Torimoto and Shuhei Ogo and Danny Harjowinoto and Takuma Higo and Seo, {Jeong Gil} and Shinya Furukawa and Yasushi Sekine",

note = "Funding Information: This work was supported by the JST CREST program and JSPS KAKENHI (grant number: 17H04965). Dr Tetsuo Honma and Dr Takeshi Watanabe (Japan Synchrotron Radiation Research Institute, SPring-8) are greatly appreciated for their kind support with XAFS measurements in BL14B2 (Proposal number: 2018A1728).",

year = "2019",

doi = "10.1039/c9cc02794g",

language = "English",

volume = "55",

pages = "6693--6695",

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T1 - Enhanced methane activation on diluted metal-metal ensembles under an electric field

T2 - Breakthrough in alloy catalysis

AU - Torimoto, Maki

AU - Ogo, Shuhei

AU - Harjowinoto, Danny

AU - Higo, Takuma

AU - Seo, Jeong Gil

AU - Furukawa, Shinya

AU - Sekine, Yasushi

N1 - Funding Information: This work was supported by the JST CREST program and JSPS KAKENHI (grant number: 17H04965). Dr Tetsuo Honma and Dr Takeshi Watanabe (Japan Synchrotron Radiation Research Institute, SPring-8) are greatly appreciated for their kind support with XAFS measurements in BL14B2 (Proposal number: 2018A1728).

PY - 2019

Y1 - 2019

N2 - Methane activation on diluted metal ensembles is a challenging task in the field of alloy chemistry. This report describes that synergy between an electric field and Pd-Zn alloy allows improved catalytic activities in the steam reforming of methane. Because of surface protonics, Pd-Pd ensembles are no longer needed. Ligand effects facilitate methane conversion.

AB - Methane activation on diluted metal ensembles is a challenging task in the field of alloy chemistry. This report describes that synergy between an electric field and Pd-Zn alloy allows improved catalytic activities in the steam reforming of methane. Because of surface protonics, Pd-Pd ensembles are no longer needed. Ligand effects facilitate methane conversion.

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