High-resolution high energy X-ray diffraction studies of charge ordering in CMR manganites and nickelates

S. B. Wilkins, P. D. Hatton, K. D. Liss, M. Ohler, Takuro Katsufuji, S. W. Cheong

Research output: Contribution to journalArticle

3 Citations (Scopus)

Abstract

High-resolution, high-energy, X-ray diffraction results are presented for the study of weak charge ordering phenomenon. By utilizing X-rays in the 100 keV region the dramatic increase in the penetration depth allows for both bulk-sensitive and high- resolution measurements to be made. The strontium doped La2NiO4 system is a prototypical system in the understanding of strong electron-phonon coupling, and the resultant effects on material properties. At doping levels of 1/3 and 1/2 commensurate charge modulations are observed indicating real-space charge stripes. We have measured the correlation lengths of these charge stripes using both 1013 keV X-rays and 8.3 keV X-rays. In comparing our results we have observed that the charge stripes appear to be well correlated in the near-surface region with correlation lengths ξ ≈ 2400Å. However, our bulk sensitive measurements show that the charge stripes appear in a possible stripe glass phase with a correlation length of only ξ ≈ 300Å. Our measurements on the 3D charge order manganite system Nd0.5Sr0.5MnO3 show that the charge ordering appears to be well correlated in the bulk of the sample in contrast to our nickelate results.

Original languageEnglish
Pages (from-to)3753-3758
Number of pages6
JournalInternational Journal of Modern Physics B
Volume14
Issue number29-31
Publication statusPublished - 2000 Dec 20
Externally publishedYes

Fingerprint

Manganites
X-ray Diffraction
High Energy
High Resolution
Charge
X ray diffraction
X rays
high resolution
diffraction
Strontium
x rays
Correlation Length
Electric space charge
energy
Materials properties
Doping (additives)
Modulation
strontium
space charge
Glass

ASJC Scopus subject areas

  • Physics and Astronomy (miscellaneous)
  • Condensed Matter Physics
  • Electronic, Optical and Magnetic Materials
  • Statistical and Nonlinear Physics
  • Mathematical Physics

Cite this

High-resolution high energy X-ray diffraction studies of charge ordering in CMR manganites and nickelates. / Wilkins, S. B.; Hatton, P. D.; Liss, K. D.; Ohler, M.; Katsufuji, Takuro; Cheong, S. W.

In: International Journal of Modern Physics B, Vol. 14, No. 29-31, 20.12.2000, p. 3753-3758.

Research output: Contribution to journalArticle

Wilkins, S. B. ; Hatton, P. D. ; Liss, K. D. ; Ohler, M. ; Katsufuji, Takuro ; Cheong, S. W. / High-resolution high energy X-ray diffraction studies of charge ordering in CMR manganites and nickelates. In: International Journal of Modern Physics B. 2000 ; Vol. 14, No. 29-31. pp. 3753-3758.
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