Key factor for the anti-Arrhenius low-temperature heterogeneous catalysis induced by H+ migration: H+ coverage over support

Kota Murakami, Yuta Tanaka, Ryuya Sakai, Yudai Hisai, Sasuga Hayashi, Yuta Mizutani, Takuma Higo, Shuhei Ogo, Jeong Gil Seo, Hideaki Tsuneki, Yasushi Sekine

Research output: Contribution to journalArticle

1 Citation (Scopus)

Abstract

Low-temperature heterogeneous catalytic reaction in an electric field is anticipated as a novel approach for on-demand and small-scale catalytic processes. This report quantitatively reveals the important role of proton coverage on the catalyst support for catalytic ammonia synthesis in an electric field, which shows an anti-Arrhenius behaviour.

Original languageEnglish
Pages (from-to)3365-3368
Number of pages4
JournalChemical Communications
Volume56
Issue number23
DOIs
Publication statusPublished - 2020 Mar 21

ASJC Scopus subject areas

  • Catalysis
  • Electronic, Optical and Magnetic Materials
  • Ceramics and Composites
  • Chemistry(all)
  • Surfaces, Coatings and Films
  • Metals and Alloys
  • Materials Chemistry

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