Low-temperature dry reforming of methane to produce syngas in an electric field over La-doped Ni/ZrO2catalysts

Tomohiro Yabe; Kenta Mitarai; Kazumasa Oshima; Shuhei Ogo; Yasushi Sekine

doi:10.1016/j.fuproc.2016.11.013

Low-temperature dry reforming of methane to produce syngas in an electric field over La-doped Ni/ZrO₂catalysts

Tomohiro Yabe, Kenta Mitarai, Kazumasa Oshima, Shuhei Ogo, Yasushi Sekine^*

^*Corresponding author for this work

School of Advanced Science and Engineering

Research output: Contribution to journal › Article › peer-review

80 Citations (Scopus)

Abstract

Dry reforming of methane (DRM) was conducted over various transition metal supported ZrO₂catalysts in an electric field. Catalyst of 1wt%Ni/10 mol%La-ZrO₂showed high DRM activity even at 423 K of external temperature, at which no DRM proceeds in the conventional catalytic systems. By virtue of the low reaction temperature, low amounts of carbon deposition were confirmed even in conditions of high CH₄conversion in the electric field. The imposed electric power was correlated to with the catalytic activities in the electric field. Syngas is producible at low temperature with high energy efficiency.

Original language	English
Pages (from-to)	96-103
Number of pages	8
Journal	Fuel Processing Technology
Volume	158
DOIs	https://doi.org/10.1016/j.fuproc.2016.11.013
Publication status	Published - 2017

Keywords

Carbon dioxide utilization
Dry reforming of methane
Electric field
Low carbon deposition
Low temperature catalytic reaction

ASJC Scopus subject areas

Chemical Engineering(all)
Fuel Technology
Energy Engineering and Power Technology

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1016/j.fuproc.2016.11.013

Cite this

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title = "Low-temperature dry reforming of methane to produce syngas in an electric field over La-doped Ni/ZrO2catalysts",

abstract = "Dry reforming of methane (DRM) was conducted over various transition metal supported ZrO2catalysts in an electric field. Catalyst of 1wt%Ni/10 mol%La-ZrO2showed high DRM activity even at 423 K of external temperature, at which no DRM proceeds in the conventional catalytic systems. By virtue of the low reaction temperature, low amounts of carbon deposition were confirmed even in conditions of high CH4conversion in the electric field. The imposed electric power was correlated to with the catalytic activities in the electric field. Syngas is producible at low temperature with high energy efficiency.",

keywords = "Carbon dioxide utilization, Dry reforming of methane, Electric field, Low carbon deposition, Low temperature catalytic reaction",

author = "Tomohiro Yabe and Kenta Mitarai and Kazumasa Oshima and Shuhei Ogo and Yasushi Sekine",

note = "Publisher Copyright: {\textcopyright} 2016 Elsevier B.V.",

year = "2017",

doi = "10.1016/j.fuproc.2016.11.013",

language = "English",

volume = "158",

pages = "96--103",

journal = "Fuel Processing Technology",

issn = "0378-3820",

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TY - JOUR

T1 - Low-temperature dry reforming of methane to produce syngas in an electric field over La-doped Ni/ZrO2catalysts

AU - Yabe, Tomohiro

AU - Mitarai, Kenta

AU - Oshima, Kazumasa

AU - Ogo, Shuhei

AU - Sekine, Yasushi

PY - 2017

Y1 - 2017

N2 - Dry reforming of methane (DRM) was conducted over various transition metal supported ZrO2catalysts in an electric field. Catalyst of 1wt%Ni/10 mol%La-ZrO2showed high DRM activity even at 423 K of external temperature, at which no DRM proceeds in the conventional catalytic systems. By virtue of the low reaction temperature, low amounts of carbon deposition were confirmed even in conditions of high CH4conversion in the electric field. The imposed electric power was correlated to with the catalytic activities in the electric field. Syngas is producible at low temperature with high energy efficiency.

AB - Dry reforming of methane (DRM) was conducted over various transition metal supported ZrO2catalysts in an electric field. Catalyst of 1wt%Ni/10 mol%La-ZrO2showed high DRM activity even at 423 K of external temperature, at which no DRM proceeds in the conventional catalytic systems. By virtue of the low reaction temperature, low amounts of carbon deposition were confirmed even in conditions of high CH4conversion in the electric field. The imposed electric power was correlated to with the catalytic activities in the electric field. Syngas is producible at low temperature with high energy efficiency.

KW - Carbon dioxide utilization

KW - Dry reforming of methane

KW - Electric field

KW - Low carbon deposition

KW - Low temperature catalytic reaction

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