Microwave conductivity of superconducting and insulating fullerides

H. Kitano, R. Matsuo, K. Miwa, A. Maeda, T. Takenobu, Y. Iwasa

Research output: Contribution to journalArticle

2 Citations (Scopus)

Abstract

Superconductivity of A3 C60 (A = K and Rb) is destroyed by the intercalation of neutral ammonia molecules, and is replaced by the antiferromagnetic ground state. These properties suggest the importance of the electronic correlation in fullerides, which have been believed to be simple BCS superconductors. By using a microwave cavity perturbation technique, we confirmed that the conductivity of the antiferromagnet (NH3) K3-x Rbx C60 at 200K is already 3-4 orders of magnitude smaller than those of superconductors, K3 C60 and (NH3)x NaRb2 C60, and that the antiferromagnetic compounds are insulators without metal-insulator transition at the Néel temperature. These results indicate that the Mott-Hubbard transition in the A3 C60 systems is driven by a reduction of lattice symmetry from face-centered-cubic (fcc) to face-centered-orthorhombic (fco), rather than by the magnetic ordering.

Original languageEnglish
Pages (from-to)1251-1258
Number of pages8
JournalJournal of Low Temperature Physics
Volume131
Issue number5-6
DOIs
Publication statusPublished - 2003 Jun
Externally publishedYes

Fingerprint

fullerides
Superconducting materials
Microwaves
insulators
microwaves
conductivity
Perturbation techniques
Metal insulator transition
Intercalation
Superconductivity
Ammonia
intercalation
Ground state
ammonia
Magnetization
superconductivity
perturbation
cavities
Molecules
ground state

ASJC Scopus subject areas

  • Physics and Astronomy (miscellaneous)

Cite this

Kitano, H., Matsuo, R., Miwa, K., Maeda, A., Takenobu, T., & Iwasa, Y. (2003). Microwave conductivity of superconducting and insulating fullerides. Journal of Low Temperature Physics, 131(5-6), 1251-1258. https://doi.org/10.1023/A:1023450521090

Microwave conductivity of superconducting and insulating fullerides. / Kitano, H.; Matsuo, R.; Miwa, K.; Maeda, A.; Takenobu, T.; Iwasa, Y.

In: Journal of Low Temperature Physics, Vol. 131, No. 5-6, 06.2003, p. 1251-1258.

Research output: Contribution to journalArticle

Kitano, H, Matsuo, R, Miwa, K, Maeda, A, Takenobu, T & Iwasa, Y 2003, 'Microwave conductivity of superconducting and insulating fullerides', Journal of Low Temperature Physics, vol. 131, no. 5-6, pp. 1251-1258. https://doi.org/10.1023/A:1023450521090
Kitano, H. ; Matsuo, R. ; Miwa, K. ; Maeda, A. ; Takenobu, T. ; Iwasa, Y. / Microwave conductivity of superconducting and insulating fullerides. In: Journal of Low Temperature Physics. 2003 ; Vol. 131, No. 5-6. pp. 1251-1258.
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