Observation of Plasmon Wave Packet Motions via Femtosecond Time-Resolved Near-Field Imaging Techniques

Yoshio Nishiyama, Kohei Imura, Hiromi Okamoto

Research output: Contribution to journalArticlepeer-review

19 Citations (Scopus)

Abstract

The generation and dynamics of plasmon wave packets in single gold nanorods were observed at a spatiotemporal scale of 100 nm and 10 fs via time-resolved near-field optical microscopy. Following simultaneous excitation of two plasmon modes of a nanorod with an ultrashort near-field pulse, a decay and revival feature of the time-resolved signal was obtained, which reflected the reciprocating motion of the wave packet. The time-resolved near-field images were also indicative of the wave packet motion. At some period of time after the excitation, the spatial features of the two modes appeared alternately, showing motion of plasmonic wave crests along the rod. The wave packet propagation was clearly demonstrated from this observation with the aid of a simulation model. The present experimental scheme opens the door to coherent control of plasmon-induced optical fields in a nanometer spatial scale and femtosecond temporal scale.

Original languageEnglish
Pages (from-to)7657-7665
Number of pages9
JournalNano Letters
Volume15
Issue number11
DOIs
Publication statusPublished - 2015 Nov 11

Keywords

  • Plasmon wave packet
  • nanoscale
  • near-field optical microscopy
  • ultrafast dynamics

ASJC Scopus subject areas

  • Bioengineering
  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanical Engineering

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