Single crystal-like selection rules for unipolar-axis oriented tetragonal Pb (Zr,Ti) O3 thick epitaxial films

Mitsumasa Nakajima, Takashi Fujisawa, Yoshitaka Ehara, Tomoaki Yamada, Hiroshi Funakubo, Hiroshi Naganuma, Soichiro Okamura, Ken Nishida, Takashi Yamamoto, Minoru Osada

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Abstract

We investigated the polarized Raman spectra of a strain-free, unipolar-axis oriented tetragonal Pb (Zr,Ti) O3 thick epitaxial film. We evaluated the single crystal-like selection rules of the A1-and E-symmetry components, and found an anomalous behavior in the angular dependence of the A1 (1TO)-mode intensity similar to that observed in high-T c superconductor single crystals. Raman tensor analyses of the A 1 (1TO) mode revealed complex phases may exist between two independent Raman-tensor components even in the single 180° domain state.

Original languageEnglish
Article number111901
JournalApplied Physics Letters
Volume97
Issue number11
DOIs
Publication statusPublished - 2010 Sep 13
Externally publishedYes

ASJC Scopus subject areas

  • Physics and Astronomy (miscellaneous)

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    Nakajima, M., Fujisawa, T., Ehara, Y., Yamada, T., Funakubo, H., Naganuma, H., Okamura, S., Nishida, K., Yamamoto, T., & Osada, M. (2010). Single crystal-like selection rules for unipolar-axis oriented tetragonal Pb (Zr,Ti) O3 thick epitaxial films. Applied Physics Letters, 97(11), [111901]. https://doi.org/10.1063/1.3488015