Studying the electronic structure of molecules with high harmonic spectroscopy

D. M. Villeneuve; J. B. Bertrand; P. B. Corkum; N. Dudovich; J. Itatani; J. C. Kieffer; F. Légaré; J. Levesque; Y. Mairesse; H. Niikura; B. E. Schmidt; A. D. Shiner; H. J. Wörner

doi:10.1007/978-3-642-37623-8_10

Studying the electronic structure of molecules with high harmonic spectroscopy

D. M. Villeneuve^*, J. B. Bertrand, P. B. Corkum, N. Dudovich, J. Itatani, J. C. Kieffer, F. Légaré, J. Levesque, Y. Mairesse, H. Niikura, B. E. Schmidt, A. D. Shiner, H. J. Wörner

^*Corresponding author for this work

School of Advanced Science and Engineering

Research output: Chapter in Book/Report/Conference proceeding › Chapter

Abstract

High harmonic spectroscopy is a tool to study the valence electronic structure of atoms and molecules. It uses the techniques of high harmonic generation, in which a femtosecond laser ionizes the gas sample and XUV radiation is emitted in the forward direction. The XUV intensity, phase and polarization contain information about the orbital from which an electron was removed by the laser. High harmonic spectroscopy reveals details of electron-electron interactions, motion of electronic wave packets, and can follow a chemical reaction.

Original language	English
Title of host publication	Attosecond Physics
Subtitle of host publication	Attosecond Measurements and Control of Physical Systems
Publisher	Springer Verlag
Pages	159-190
Number of pages	32
ISBN (Print)	9783642376221
DOIs	https://doi.org/10.1007/978-3-642-37623-8_10
Publication status	Published - 2013

Publication series

Name	Springer Series in Optical Sciences
Volume	177
ISSN (Print)	0342-4111
ISSN (Electronic)	1556-1534

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials

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10.1007/978-3-642-37623-8_10

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Villeneuve, D. M., Bertrand, J. B., Corkum, P. B., Dudovich, N., Itatani, J., Kieffer, J. C., Légaré, F., Levesque, J., Mairesse, Y., Niikura, H., Schmidt, B. E., Shiner, A. D., & Wörner, H. J. (2013). Studying the electronic structure of molecules with high harmonic spectroscopy. In Attosecond Physics: Attosecond Measurements and Control of Physical Systems (pp. 159-190). (Springer Series in Optical Sciences; Vol. 177). Springer Verlag. https://doi.org/10.1007/978-3-642-37623-8_10

Studying the electronic structure of molecules with high harmonic spectroscopy. / Villeneuve, D. M.; Bertrand, J. B.; Corkum, P. B. et al.

Attosecond Physics: Attosecond Measurements and Control of Physical Systems. Springer Verlag, 2013. p. 159-190 (Springer Series in Optical Sciences; Vol. 177).

Research output: Chapter in Book/Report/Conference proceeding › Chapter

Villeneuve, DM, Bertrand, JB, Corkum, PB, Dudovich, N, Itatani, J, Kieffer, JC, Légaré, F, Levesque, J, Mairesse, Y, Niikura, H, Schmidt, BE, Shiner, AD & Wörner, HJ 2013, Studying the electronic structure of molecules with high harmonic spectroscopy. in Attosecond Physics: Attosecond Measurements and Control of Physical Systems. Springer Series in Optical Sciences, vol. 177, Springer Verlag, pp. 159-190. https://doi.org/10.1007/978-3-642-37623-8_10

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AU - Kieffer, J. C.

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AU - Levesque, J.

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AU - Niikura, H.

AU - Schmidt, B. E.

AU - Shiner, A. D.

AU - Wörner, H. J.

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AB - High harmonic spectroscopy is a tool to study the valence electronic structure of atoms and molecules. It uses the techniques of high harmonic generation, in which a femtosecond laser ionizes the gas sample and XUV radiation is emitted in the forward direction. The XUV intensity, phase and polarization contain information about the orbital from which an electron was removed by the laser. High harmonic spectroscopy reveals details of electron-electron interactions, motion of electronic wave packets, and can follow a chemical reaction.

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Studying the electronic structure of molecules with high harmonic spectroscopy

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