Synthesis and magnetic properties of linear two-coordinate monomeric diaryliron(II) complexes bearing fused-ring bulky "Rind" groups

Shun Goda, Masanori Nikai, Mikinao Ito, Daisuke Hashizume, Kohei Tamao, Atsushi Okazawa*, Norimichi Kojima, Hiroyuki Fueno, Kazuyoshi Tanaka, Yoshio Kobayashi, Tsukasa Matsuo

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

7 Citations (Scopus)

Abstract

Monomeric diaryliron(II) complexes, Fe(Rind)2, have been obtained by introducing fused-ring bulky "Rind" groups. For Fe(Eind)2, a significant orbital contribution of the Fe(II) ion due to the linear two-coordination has been determined by the highly effective magnetic moment (μeff = 5.82 μB) and the extraordinarily large internal hyperfine field (Hn = ca. 140 T) in the Mössbauer spectrum. Variable-frequency out-of-phase ac susceptibility data demonstrate an effective spin-reversal barrier of Ueff = 51.2(7) cm-1 associated with the single-ion magnet behavior.

Original languageEnglish
Pages (from-to)634-636
Number of pages3
JournalChemistry Letters
Volume45
Issue number6
DOIs
Publication statusPublished - 2016
Externally publishedYes

Keywords

  • Diaryliron(II) complex
  • Large internal hyperfine field
  • Single-ion magnet

ASJC Scopus subject areas

  • Chemistry(all)

Fingerprint

Dive into the research topics of 'Synthesis and magnetic properties of linear two-coordinate monomeric diaryliron(II) complexes bearing fused-ring bulky "Rind" groups'. Together they form a unique fingerprint.

Cite this