Auto-methanation of Carbon Dioxide

A Novel Route for Transforming CO 2 over Ni-based Catalyst

Choji Fukuhara, Sakhon Ratchahat, Yuji Suzuki, Masao Sudoh, Ryo Watanabe

研究成果: Article

1 引用 (Scopus)

抄録

CO 2 methanation over a Ni/CeO 2 catalyst was investigated under the feeding of a raw material gas containing oxygen of 110 vol % concentration. The presence of oxygen greatly improved the methanation activity and provided high methane yield, even with cutting external heating, near room temperature. This positive phenomenon was caused by the fact that hydrogen-combustion by oxygen selectively occurred on the Ni/CeO 2 catalyst, and a large amount of thermal energy was generated. We found a novel route of CO 2 methanation that can be driven without external heating, even near room temperature, which we named auto-methanation.

元の言語English
ページ(範囲)196-199
ページ数4
ジャーナルChemistry Letters
48
発行部数3
DOI
出版物ステータスPublished - 2019 1 1
外部発表Yes

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Methanation
Carbon Monoxide
Carbon Dioxide
Catalysts
Oxygen
Heating
Methane
Thermal energy
Hydrogen
Raw materials
Gases
Temperature

Keywords

    ASJC Scopus subject areas

    • Chemistry(all)

    これを引用

    Auto-methanation of Carbon Dioxide : A Novel Route for Transforming CO 2 over Ni-based Catalyst. / Fukuhara, Choji; Ratchahat, Sakhon; Suzuki, Yuji; Sudoh, Masao; Watanabe, Ryo.

    :: Chemistry Letters, 巻 48, 番号 3, 01.01.2019, p. 196-199.

    研究成果: Article

    Fukuhara, Choji ; Ratchahat, Sakhon ; Suzuki, Yuji ; Sudoh, Masao ; Watanabe, Ryo. / Auto-methanation of Carbon Dioxide : A Novel Route for Transforming CO 2 over Ni-based Catalyst. :: Chemistry Letters. 2019 ; 巻 48, 番号 3. pp. 196-199.
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