The dielectric constant of quantum paraelectric EuTiO3, which contains Eu2+ with S=7/2 spin and Ti4+, has been measured under a magnetic field. The dielectric constant shows a critical decrease at the antiferromagnetic ordering of the Eu spins at 5.5 K, as well as a substantial change under a magnetic field (by ∼7% with 1.5 T), indicating a strong coupling between the Eu spins and dielectric properties. We show that the variation of the dielectric constant is dominated by the pair correlation of the nearest-neighbor Eu spins, likely via the variation of the soft-phonon-mode frequency.
|ジャーナル||Physical Review B - Condensed Matter and Materials Physics|
|出版ステータス||Published - 2001 8 1|
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