Determination of the local structure of the Formula Presented superconductor

G. M. Pugliese, L. Simonelli, L. Tortora, G. Tomassucci, A. Iyo, H. Eisaki, T. Mizokawa, N. L. Saini*

*この研究の対応する著者

研究成果: Article査読

抄録

We have studied the local structure of Formula Presented superconductor by As Formula Presented-edge x-ray absorption fine structure measurements as a function of temperature in a wide range of hole doping (Formula Presented = 0.0 to 0.35). A substantial change in the local structure around the arsenic atom has been observed with doping. The axial As-Formula Presented bond length is found to be >Formula Presented Å, indicating that the system is in its collapsed tetragonal phase. The temperature-dependent mean square relative displacements reveal that the As-Fe bond is relatively weak in the undoped sample; however, it gets stronger with hole doping. On the other hand, the axial As-Formula Presented bond tends to get weaker in the optimally doped regime (Formula Presented = 0.25–0.35), suggesting the possible role of increased As atom displacements in the axial direction in the superconducting phase of these materials. Consistently, the arsenic height from the Fe-Fe plane shows a gradual increase in the optimally doped regime. Apart from providing a quantitative information on the local structure of Formula Presented, the results suggest a vital role of electron-lattice coupling and axial As atom displacements in the superconductivity of these iron-based materials.

本文言語English
論文番号024519
ジャーナルPhysical Review B
105
2
DOI
出版ステータスPublished - 2022 1月 1

ASJC Scopus subject areas

  • 電子材料、光学材料、および磁性材料
  • 凝縮系物理学

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