抄録
Recent trends on the direct conversion of methane, employing carbon dioxide as an oxidizing agent are reviewed. While oxidation using molecular oxygen involves the sequential oxidation of various intermediates to generate carbon dioxide and exhibits low selectivity for the desired products, methane activation using carbon dioxide as an oxidant eliminates this sequential oxidation and has considerable promise. In this context, supported metal catalysts can promote the dry reforming of methane, and structured oxide catalysts have been found to enable methane coupling to C2 products, using carbon dioxide as the oxidizing agent. This review also summarizes recent research regarding the use of nonconventional processes for methane activation in conjunction with carbon dioxide.
| 元の言語 | English |
|---|---|
| ページ（範囲） | 187-198 |
| ページ数 | 12 |
| ジャーナル | Fuel Processing Technology |
| 巻 | 181 |
| DOI | |
| 出版物ステータス | Published - 2018 12 1 |
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ASJC Scopus subject areas
- Chemical Engineering(all)
- Fuel Technology
- Energy Engineering and Power Technology
これを引用
Methane conversion using carbon dioxide as an oxidizing agent : A review. / Yabe, Tomohiro; Sekine, Yasushi.
：: Fuel Processing Technology, 巻 181, 01.12.2018, p. 187-198.研究成果: Review article
}
TY - JOUR
T1 - Methane conversion using carbon dioxide as an oxidizing agent
T2 - A review
AU - Yabe, Tomohiro
AU - Sekine, Yasushi
PY - 2018/12/1
Y1 - 2018/12/1
N2 - Recent trends on the direct conversion of methane, employing carbon dioxide as an oxidizing agent are reviewed. While oxidation using molecular oxygen involves the sequential oxidation of various intermediates to generate carbon dioxide and exhibits low selectivity for the desired products, methane activation using carbon dioxide as an oxidant eliminates this sequential oxidation and has considerable promise. In this context, supported metal catalysts can promote the dry reforming of methane, and structured oxide catalysts have been found to enable methane coupling to C2 products, using carbon dioxide as the oxidizing agent. This review also summarizes recent research regarding the use of nonconventional processes for methane activation in conjunction with carbon dioxide.
AB - Recent trends on the direct conversion of methane, employing carbon dioxide as an oxidizing agent are reviewed. While oxidation using molecular oxygen involves the sequential oxidation of various intermediates to generate carbon dioxide and exhibits low selectivity for the desired products, methane activation using carbon dioxide as an oxidant eliminates this sequential oxidation and has considerable promise. In this context, supported metal catalysts can promote the dry reforming of methane, and structured oxide catalysts have been found to enable methane coupling to C2 products, using carbon dioxide as the oxidizing agent. This review also summarizes recent research regarding the use of nonconventional processes for methane activation in conjunction with carbon dioxide.
KW - C hydrocarbon
KW - Catalytic methane conversion
KW - Electric field
KW - Endothermic reaction
KW - Syngas production
UR - http://www.scopus.com/inward/record.url?scp=85054171026&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=85054171026&partnerID=8YFLogxK
U2 - 10.1016/j.fuproc.2018.09.014
DO - 10.1016/j.fuproc.2018.09.014
M3 - Review article
AN - SCOPUS:85054171026
VL - 181
SP - 187
EP - 198
JO - Fuel Processing Technology
JF - Fuel Processing Technology
SN - 0378-3820
ER -