New method for direct conversion of methane

Y. Sekine, K. Fujimoto

研究成果: Article査読

2 被引用数 (Scopus)

抄録

Methane was oxidized by oxygen in the absence of a catalyst with the microwire initiation (MWI) method, which was composed of an electrically heated small wire and a low-temperature reaction zone. With the existence of initiation reaction, methanol and carbon monoxide were formed at 393 K gas phase temperature. The main products of the reaction were methanol, hydrogen, carbon monoxide, carbon dioxide, and water. With the batch-wise MWI system, methanol selectivity was higher than 80% at the initial stage of the reaction. In the absence of MWI, no products were formed under 653 K of gas phase temperature in the chain reaction zone. We proposed a new model for the oxidation of methane with microwire initiation.

本文言語English
ページ(範囲)294-300
ページ数7
ジャーナルKinetics and Catalysis
40
3
出版ステータスPublished - 1999 5 1
外部発表はい

ASJC Scopus subject areas

  • 触媒
  • 化学 (全般)
  • モデリングとシミュレーション
  • コンピュータ サイエンスの応用

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