Optical freezing of charge motion in an organic conductor

Takahiro Ishikawa, Yuto Sagae, Yota Naitoh, Yohei Kawakami, Hirotake Itoh, Kaoru Yamamoto, Kyuya Yakushi, Hideo Kishida, Takahiko Sasaki, Sumio Ishihara, Yasuhiro Tanaka, Kenji Yonemitsu, Shinichiro Iwai*

*この研究の対応する著者

研究成果: Article査読

45 被引用数 (Scopus)

抄録

Dynamical localization, that is, reduction of the intersite electronic transfer integral t by an alternating electric field, E(ω), is a promising strategy for controlling strongly correlated systems with a competing energy balance between t and the Coulomb repulsion energy. Here we describe a charge localization induced by the 9.3 MV cm-1 instantaneous electric field of a 1.5 cycle (7 fs) infrared pulse in an organic conductor α-(bis[ethylenedithio]-tetrathiafulvalene)2I3. A large reflectivity change of >25% and a coherent charge oscillation along the time axis reflect the opening of the charge ordering gap in the metallic phase. This optical freezing of charges, which is the reverse of the photoinduced melting of electronic orders, is attributed to the ∼10% reduction of t driven by the strong, high-frequency (ω≥ t/H) electric field.

本文言語English
論文番号5528
ジャーナルNature communications
5
DOI
出版ステータスPublished - 2014
外部発表はい

ASJC Scopus subject areas

  • 化学 (全般)
  • 生化学、遺伝学、分子生物学(全般)
  • 物理学および天文学(全般)

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