TY - JOUR
T1 - Orbital-spin structure and lattice coupling in [formula presented] where [formula presented], [formula presented], [formula presented], and [formula presented]
AU - Mochizuki, Masahito
AU - Imada, Masatoshi
PY - 2003/1/1
Y1 - 2003/1/1
N2 - The origin of the G-type antiferromagnetism [AFM(G)] and puzzling properties of [Formula presented] with [Formula presented] are studied. We clarify that the crystal field from La caused by the [Formula presented]-type distortion lifts the [Formula presented] degeneracy at Ti [Formula presented] orbitals. The lift stabilizes the AFM(G) with spin-exchange constant in agreement with neutron-scattering results. The orbital-spin structures for [Formula presented], Nd, and Sm are also consistent with experiments. We propose that the [Formula presented]-type distortion has a universal mechanism of controlling orbital-spin structure competing with the Jahn-Teller (JT) mechanism.
AB - The origin of the G-type antiferromagnetism [AFM(G)] and puzzling properties of [Formula presented] with [Formula presented] are studied. We clarify that the crystal field from La caused by the [Formula presented]-type distortion lifts the [Formula presented] degeneracy at Ti [Formula presented] orbitals. The lift stabilizes the AFM(G) with spin-exchange constant in agreement with neutron-scattering results. The orbital-spin structures for [Formula presented], Nd, and Sm are also consistent with experiments. We propose that the [Formula presented]-type distortion has a universal mechanism of controlling orbital-spin structure competing with the Jahn-Teller (JT) mechanism.
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U2 - 10.1103/PhysRevLett.91.167203
DO - 10.1103/PhysRevLett.91.167203
M3 - Article
AN - SCOPUS:84904264807
VL - 91
JO - Physical Review Letters
JF - Physical Review Letters
SN - 0031-9007
IS - 16
ER -