Signature of Kondo hybridisation with an orbital-selective Mott phase in 4d Ca2−xSrxRuO4

Minsoo Kim, Junyoung Kwon, Choong H. Kim, Younsik Kim, Daun Chung, Hanyoung Ryu, Jongkeun Jung, Beom Seo Kim, Dongjoon Song, Jonathan D. Denlinger, Moonsup Han, Yoshiyuki Yoshida, Takashi Mizokawa, Wonshik Kyung*, Changyoung Kim

*この研究の対応する著者

研究成果: Article査読

抄録

The heavy fermion state with Kondo-hybridisation (KH), usually manifested in f-electron systems with lanthanide or actinide elements, was recently discovered in several 3d transition metal compounds without f-electrons. However, KH has not yet been observed in 4d/5d transition metal compounds, since more extended 4d/5d orbitals do not usually form flat bands that supply localised electrons appropriate for Kondo pairing. Here, we report a substitution- and temperature-dependent angle-resolved photoemission study on 4d Ca2−xSrxRuO4, which shows the signature of KH. We observed a spectral weight transfer in the γ-band, reminiscent of an orbital-selective Mott phase (OSMP). The Mott localised γ-band induces the KH with an itinerant β-band, resulting in spectral weight suppression around the Fermi level. Our work demonstrates the evolution of the OSMP with possible KH among 4d electrons, and thereby expands the material boundary of Kondo physics to 4d multi-orbital systems.

本文言語English
論文番号59
ジャーナルnpj Quantum Materials
7
1
DOI
出版ステータスPublished - 2022 12月

ASJC Scopus subject areas

  • 電子材料、光学材料、および磁性材料
  • 凝縮系物理学

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