Spatiotemporal variations of fine particulate organic and elemental carbons in Greater Tokyo

Hiroshi Hayami*, Shinji Saito, Shuichi Hasegawa

*この研究の対応する著者

研究成果: Article査読

2 被引用数 (Scopus)

抄録

Hourly concentrations of fine particulate OC and EC are monitored for more than one year by optical monitors at three sites in and out of Tokyo, Japan. Distances between the sites are 20 to 50 km. SOC concentrations are estimated from the OC and EC concentrations by an EC tracer method. Site A in an industrial site shows higher EC concentrations than site B in a residential area, but differences between the sites are much reduced for OC. Site C in a rural area, where measurements are available in colder months, shows pronounced seasonal variations with high peaks in October and December and characteristic diurnal variations in OC with the highest in the evening in October, due probably to open field burning. Photochemical formation of SOC is suggested but does not rise up so much OC concentrations in summer, which are quite lower than other seasons. A comparison between relative concentrations of EC among the sites and local emissions amounts indicates missing or considerable underestimation of EC emissions near the rural site C. Time lag correlations suggest transport of OC produced by open field burning around site C to site A. These findings would be useful for improving model performances in OC/EC predictions.

本文言語English
ページ(範囲)161-170
ページ数10
ジャーナルAsian Journal of Atmospheric Environment
13
3
DOI
出版ステータスPublished - 2019
外部発表はい

ASJC Scopus subject areas

  • 環境科学(全般)
  • 大気科学

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